Electrochemical Oscillatory Baffled Reactors Fabricated with Additive Manufacturing for Efficient Continuous-Flow Oxidations
Impacto
Scholar |
Otros documentos de la autoría: Alvarez, Elena; Romero-Fernandez, Maria; Iglesias, Diego; Martinez Cuenca, Raul; Okafor, Obinna; Delorme, Astrid E.; Lozano, Pedro; Goodridge, Ruth; Paradisi, Francesca; Walsh, Darren; Sans, Victor
Metadatos
Mostrar el registro completo del ítemcomunitat-uji-handle:10234/9
comunitat-uji-handle2:10234/160292
comunitat-uji-handle3:10234/160293
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INVESTIGACIONMetadatos
Título
Electrochemical Oscillatory Baffled Reactors Fabricated with Additive Manufacturing for Efficient Continuous-Flow OxidationsAutoría
Fecha de publicación
2022-02-21Editor
American Chemical SocietyISSN
2168-0485Cita bibliográfica
Alvarez, E.; Romero-Fernandez, M.; Iglesias, D.; Martinez-Cuenca, R.; Okafor, O.; Delorme, A.; Lozano, P.; Goodridge, R.; Paradisi, F.; Walsh, Darren A.; Sans, V. Electrochemical Oscillatory Baffled Reactors Fabricated with Additive Manufacturing for Efficient Continuous-Flow Oxidations. ACS Sustainable Chem. Eng. 2022, 10, 7, 2388–2396. DOI: 10.1021/acssuschemeng.1c06799Tipo de documento
info:eu-repo/semantics/articleVersión de la editorial
https://pubs.acs.org/doi/10.1021/acssuschemeng.1c06799Versión
info:eu-repo/semantics/publishedVersionPalabras clave / Materias
Resumen
Electrochemical continuous-flow reactors offer a great opportunity for enhanced and sustainable chemical syntheses. Here, we present a novel application of electrochemical continuous-flow oscillatory baffled reactors ... [+]
Electrochemical continuous-flow reactors offer a great opportunity for enhanced and sustainable chemical syntheses. Here, we present a novel application of electrochemical continuous-flow oscillatory baffled reactors (ECOBRs) that combines advanced mixing features with electrochemical transformations to enable efficient electrochemical oxidations under continuous flow at a millimeter distance between electrodes. Different additive manufacturing techniques have been employed to rapidly fabricate reactors. The electrochemical oxidation of NADH, a very sensitive substrate key for the regeneration of enzymes in biocatalytic transformations, has been employed as a benchmark reaction. The oscillatory conditions improved bulk mixing, facilitating the contact of reagents to electrodes. Under oscillatory conditions, the ECOBR demonstrated improved performance in the electrochemical oxidation of NADH, which is attributed to improved mass transfer associated with the oscillatory regime. [-]
Publicado en
ACS Sustainable Chem. Eng. 2022, 10, 7, 2388–2396Datos relacionados
https://pubs.acs.org/doi/10.1021/acssuschemeng.1c06799?goto=supporting-infoEntidad financiadora
Generalitat Valenciana | Ministerio de Ciencia, Innovación y Universidades | Fundación SENECA CARM | University Jaume I | European Commission | Biotechnology and Biological Sciences Research Council | EPSRC CDT in Sustainable Chemistry
Identificador de la entidad financiadora
http://dx.doi.org/10.13039/501100011033
Código del proyecto o subvención
CIDEGENT/2018/036 | MICIU/ICTI2017-2020/PID2020-119628RB-C33 | MICIU/ICTI2017-2020/RTI2018-098233-B-C21 | 20790/PI/18 | UJI-B2016-52 | info:eu-repo/grantAgreement/EC/H2020/722361 | BB/R021287/1 | EP/L015633/1
Título del proyecto o subvención
Fabricación avanzada para procesos de cristalización de perovskitas | Nuevos procesos multi-catalíticos verdes basados en la tecnología de los líquidos iónicos. Desde las materias primas sencillas hasta los productos químicos con valor añadido
Derechos de acceso
Copyright © 2022 The Authors. Published by American Chemical Society
info:eu-repo/semantics/openAccess
info:eu-repo/semantics/openAccess
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- INAM_Articles [521]