Electrochemical Oscillatory Baffled Reactors Fabricated with Additive Manufacturing for Efficient Continuous-Flow Oxidations
Impacte
Scholar |
Altres documents de l'autoria: Alvarez, Elena; Romero-Fernandez, Maria; Iglesias, Diego; Martinez Cuenca, Raul; Okafor, Obinna; Delorme, Astrid E.; Lozano, Pedro; Goodridge, Ruth; Paradisi, Francesca; Walsh, Darren; Sans, Victor
Metadades
Mostra el registre complet de l'elementcomunitat-uji-handle:10234/9
comunitat-uji-handle2:10234/160292
comunitat-uji-handle3:10234/160293
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INVESTIGACIONMetadades
Títol
Electrochemical Oscillatory Baffled Reactors Fabricated with Additive Manufacturing for Efficient Continuous-Flow OxidationsAutoria
Data de publicació
2022-02-21Editor
American Chemical SocietyISSN
2168-0485Cita bibliogràfica
Alvarez, E.; Romero-Fernandez, M.; Iglesias, D.; Martinez-Cuenca, R.; Okafor, O.; Delorme, A.; Lozano, P.; Goodridge, R.; Paradisi, F.; Walsh, Darren A.; Sans, V. Electrochemical Oscillatory Baffled Reactors Fabricated with Additive Manufacturing for Efficient Continuous-Flow Oxidations. ACS Sustainable Chem. Eng. 2022, 10, 7, 2388–2396. DOI: 10.1021/acssuschemeng.1c06799Tipus de document
info:eu-repo/semantics/articleVersió de l'editorial
https://pubs.acs.org/doi/10.1021/acssuschemeng.1c06799Versió
info:eu-repo/semantics/publishedVersionParaules clau / Matèries
Resum
Electrochemical continuous-flow reactors offer a great opportunity for enhanced and sustainable chemical syntheses. Here, we present a novel application of electrochemical continuous-flow oscillatory baffled reactors ... [+]
Electrochemical continuous-flow reactors offer a great opportunity for enhanced and sustainable chemical syntheses. Here, we present a novel application of electrochemical continuous-flow oscillatory baffled reactors (ECOBRs) that combines advanced mixing features with electrochemical transformations to enable efficient electrochemical oxidations under continuous flow at a millimeter distance between electrodes. Different additive manufacturing techniques have been employed to rapidly fabricate reactors. The electrochemical oxidation of NADH, a very sensitive substrate key for the regeneration of enzymes in biocatalytic transformations, has been employed as a benchmark reaction. The oscillatory conditions improved bulk mixing, facilitating the contact of reagents to electrodes. Under oscillatory conditions, the ECOBR demonstrated improved performance in the electrochemical oxidation of NADH, which is attributed to improved mass transfer associated with the oscillatory regime. [-]
Publicat a
ACS Sustainable Chem. Eng. 2022, 10, 7, 2388–2396Dades relacionades
https://pubs.acs.org/doi/10.1021/acssuschemeng.1c06799?goto=supporting-infoEntitat finançadora
Generalitat Valenciana | Ministerio de Ciencia, Innovación y Universidades | Fundación SENECA CARM | University Jaume I | European Commission | Biotechnology and Biological Sciences Research Council | EPSRC CDT in Sustainable Chemistry
Identificador de l'entitat finançadora
http://dx.doi.org/10.13039/501100011033
Codi del projecte o subvenció
CIDEGENT/2018/036 | MICIU/ICTI2017-2020/PID2020-119628RB-C33 | MICIU/ICTI2017-2020/RTI2018-098233-B-C21 | 20790/PI/18 | UJI-B2016-52 | info:eu-repo/grantAgreement/EC/H2020/722361 | BB/R021287/1 | EP/L015633/1
Títol del projecte o subvenció
Fabricación avanzada para procesos de cristalización de perovskitas | Nuevos procesos multi-catalíticos verdes basados en la tecnología de los líquidos iónicos. Desde las materias primas sencillas hasta los productos químicos con valor añadido
Drets d'accés
Copyright © 2022 The Authors. Published by American Chemical Society
info:eu-repo/semantics/openAccess
info:eu-repo/semantics/openAccess
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