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Perovskite Thin Single Crystal for a High Performance and Long Endurance Memristor
dc.contributor.author | Fernandez-Guillen, Ismael | |
dc.contributor.author | Aranda Alonso, Clara | |
dc.contributor.author | Franco Betancur, Pablo | |
dc.contributor.author | Vallés-Pelarda, Marta | |
dc.contributor.author | Momblona, Cristina | |
dc.contributor.author | Ripolles, Teresa S. | |
dc.contributor.author | Abargues, Rafael | |
dc.contributor.author | Boix, Pablo P | |
dc.date.accessioned | 2024-04-19T12:31:39Z | |
dc.date.available | 2024-04-19T12:31:39Z | |
dc.date.issued | 2024 | |
dc.identifier.citation | I. Fernandez-Guillen, C. A. Aranda, P. F. Betancur, M. Vallés-Pelarda, C. Momblona, T. S. Ripolles, R. Abargues, P. P. Boix, Perovskite Thin Single Crystal for a High Performance and Long Endurance Memristor. Adv. Electron. Mater. 2024, 2300475. https://doi.org/10.1002/aelm.202300475 | ca_CA |
dc.identifier.issn | 2199-160X | |
dc.identifier.uri | http://hdl.handle.net/10234/206488 | |
dc.description.abstract | Metal halide perovskites (MHPs) exhibit electronic and ionic characteristics suitable for memristors. However, polycrystalline thin film perovskite memristors often suffer from reliability issues due to grain boundaries, while bulk single-crystal perovskite memristors struggle to achieve high LRS/HRS ratios. In this study, a single crystal memristive device utilizing a wide bandgap perovskite is introduced, MAPbBr3, in a high surface/thickness configuration. This thin single crystal overcomes these challenges, exhibiting a remarkable LRS/HRS ratio of up to 50 and endurance of 103 cycles, representing one of the highest reported values to date. This exceptional stability enables to analyze the electroforming process and LRS through impedance spectroscopy, providing insights into the underlying operational mechanism. As far as it is known, this is the first reported thin single-crystal MHP memristor device and the first time that the electroforming process is recorded through impedance spectroscopy. This device's outstanding stability and performance position it as a promising candidate for high-density data storage and neuromorphic applications. | ca_CA |
dc.format.extent | 12 p. | ca_CA |
dc.format.mimetype | application/pdf | ca_CA |
dc.language.iso | eng | ca_CA |
dc.publisher | Wiley | ca_CA |
dc.relation | Perovskitas de metal haluro: nuevas estructuras para nuevos retos | ca_CA |
dc.relation.isPartOf | Advanced Electronic Materials, 2024 | ca_CA |
dc.rights | © 2024 The Authors. Advanced Electronic Materials published by Wiley-VCH GmbH. This is an open access article under the terms of the Creative Commons Attribution License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited | ca_CA |
dc.rights.uri | http://creativecommons.org/licenses/by/4.0/ | ca_CA |
dc.subject | electroforming | ca_CA |
dc.subject | endurance | ca_CA |
dc.subject | impedance spectroscopy | ca_CA |
dc.subject | memristors | ca_CA |
dc.subject | perovskite | ca_CA |
dc.title | Perovskite Thin Single Crystal for a High Performance and Long Endurance Memristor | ca_CA |
dc.type | info:eu-repo/semantics/article | ca_CA |
dc.identifier.doi | https://doi.org/10.1002/aelm.202300475 | |
dc.rights.accessRights | info:eu-repo/semantics/openAccess | ca_CA |
dc.relation.publisherVersion | https://onlinelibrary.wiley.com/doi/full/10.1002/aelm.202300475 | ca_CA |
dc.description.sponsorship | C.A.A was supported by the Margarita Salas postdoctoral contract MGS/2021/24(UP2021-021) financed by the European Union-NextGenerationEU. The authors would like to acknowledge the funding by MCIN/ AEI /10.13039/501100011033 (Research project no. PID2020-119628RB-C31). PPB and TR thank Generalitat Valenciana for the funding via Pla Gent-T (grants CIDEXG/2022/34). C.M. acknowledges the funding from the “Contratación de personal investigador doctor con experiencia internacional CDEIGENT” (ref CDEIGENT/2021/2022) from the Consellería de Innovación, Universidades, Ciencia y Sociedad Digital de la Generalitat Valenciana, Spain.This study forms part of the Advanced Materials programme and was supported by MCIN with funding from European Union NextGenerationEU (PRTR-C17.I1) and by the Generalitat Valenciana (code MFA/2022/040 /007). The work was partially funded by MCIN/ AEI through project TED2021-131600B-C32. | |
dc.type.version | info:eu-repo/semantics/publishedVersion | ca_CA |
project.funder.identifier | http://dx.doi.org/10.13039/501100011033 | ca_CA |
project.funder.name | European Union | ca_CA |
project.funder.name | Ministerio de Ciencia, Innovación y Universidades | ca_CA |
project.funder.name | Generalitat Valenciana | ca_CA |
project.funder.name | Ministerio de Ciencia e Innovación | ca_CA |
oaire.awardNumber | MGS/2021/24(UP2021‐021) | ca_CA |
oaire.awardNumber | MICIU/ICTI2017-2020/PID2020-119628RB-C31) | ca_CA |
oaire.awardNumber | CIDEXG/2022/34 | ca_CA |
oaire.awardNumber | CDEIGENT/2021/2022 | ca_CA |
oaire.awardNumber | MFA/2022/040 /007 | ca_CA |
oaire.awardNumber | MCIN/PEICTI2021-2023/TED2021-131600B-C32 | ca_CA |
dc.subject.ods | 7. Energia asequible y no contaminante | ca_CA |
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