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A Perovskite Photovoltaic Mini-Module-CsPbBr3 Photoelectrochemical Cell Tandem Device for Solar-Driven Degradation of Organic Compounds
| dc.contributor.author | Lee, Seul-Yi | |
| dc.contributor.author | Serafini, Patricio | |
| dc.contributor.author | Masi, Sofia | |
| dc.contributor.author | Gualdrón Reyes, Andrés Fabián | |
| dc.contributor.author | Mesa, Camilo A. | |
| dc.contributor.author | Rodriguez-Pereira, Jhonatan | |
| dc.contributor.author | Gimenez, Sixto | |
| dc.contributor.author | Lee, Hyo Joong | |
| dc.contributor.author | Mora-Sero, Ivan | |
| dc.date.accessioned | 2023-12-01T13:37:29Z | |
| dc.date.available | 2023-12-01T13:37:29Z | |
| dc.date.issued | 2023-10-02 | |
| dc.identifier.citation | Lee, S. Y., Serafini, P., Masi, S., Gualdrón-Reyes, A. F., Mesa, C. A., Rodríguez-Pereira, J., Gimenez, S.,Lee, H. J., Mora-Seró, I. A Perovskite Photovoltaic Mini-Module-CsPbBr<sub>3</sub> Photoelectrochemical Cell Tandem Device for Solar-Driven Degradation of Organic Compounds. ACS Energy Lett. 2023, 8, 10, 4488-4495 DOI: 10.1021/acsenergylett.3c01361 | ca_CA |
| dc.identifier.issn | 2380-8195 | |
| dc.identifier.uri | http://hdl.handle.net/10234/205098 | |
| dc.description.abstract | Recently, halide perovskites have been widely explored for high-efficiency photocatalysis or photoelectrochemical (PEC) cells. Here, in order to make an efficient photoanode electrode for the degradation of pollutants, concretely 2-mercaptobenzothiazole (MBT), nanoscale cesium lead bromide (CsPbBr3) perovskite was directly formed on the surface of mesoporous titanium dioxide (meso-TiO2) film using a two-step spin-coating process. This photoelectrode recorded a photocurrent of up to 3.02 ± 0.03 mA/cm2 under standard AM 1.5G (100 mW/cm2) illumination through an optimization process such as introducing a thin aluminum oxide (Al2O3) coating layer. Furthermore, to supply high voltage for efficient oxidation of MBT without an external bias, we developed a new photovoltaic/PEC tandem system using a methylammonium lead iodide (MAPbI3) based mini-module consisting of three solar cells interconnected in series and confirmed its successful operation. This approach looks very promising due to its applicability to various PEC reactions. | ca_CA |
| dc.description.sponsorShip | Funding for open access charge: CRUE-Universitat Jaume I | |
| dc.format.extent | 8 p. | ca_CA |
| dc.format.mimetype | application/pdf | ca_CA |
| dc.language.iso | eng | ca_CA |
| dc.publisher | American Chemical Society | ca_CA |
| dc.relation.isPartOf | ACS Energy Letters, 2023, vol. 8, no 10 | ca_CA |
| dc.rights.uri | http://creativecommons.org/licenses/by/4.0/ | ca_CA |
| dc.subject | halide perovskites | ca_CA |
| dc.subject | perovskite solar cells | ca_CA |
| dc.subject | degradation of organic compounds | ca_CA |
| dc.title | A Perovskite Photovoltaic Mini-Module-CsPbBr3 Photoelectrochemical Cell Tandem Device for Solar-Driven Degradation of Organic Compounds | ca_CA |
| dc.type | info:eu-repo/semantics/article | ca_CA |
| dc.identifier.doi | https://doi.org/10.1021/acsenergylett.3c01361 | |
| dc.rights.accessRights | info:eu-repo/semantics/openAccess | ca_CA |
| dc.relation.publisherVersion | https://pubs.acs.org/doi/full/10.1021/acsenergylett.3c01361 | ca_CA |
| dc.description.sponsorship | This research was supported by Basic Science Research Program through the National Research Foundation of Korea (NRF) funded by the Ministry of Education (2022R1A6A3A03068188 & 2022R1A2C1008252). The authors also thank Generalitat Valenciana via Prometeo Grant Q-Solutions (CIPROM/2021/078) and Next Generation EU Advanced Materials Grant Print-P (MFA/2022/020), Project She-LED PID2021-122960OA-I00 funded by MCIN/AEI/10.13039/501100011033/and by FEDER, Project Step-Up (TED2021-131600B–C31) funded by Ministry of Science and Technology (Spain), and the Ministry of Education, Youth and Sports of the Czech Republic, for the financial support of XPS measurements using the CEMNAT infrastructure (project LM 2018103 and LM2023037). C.A.M. acknowledges the Generalitat Valenciana for funding through the APOSTD/2021/251 fellowship. S.M. acknowledges financial support from MICINN (Spain) through the program Juan de la Cierva-Incorporatión IJC2020-042618-I. | |
| dc.type.version | info:eu-repo/semantics/publishedVersion | ca_CA |
| project.funder.name | National Research Foundation of Korea (NRF) | ca_CA |
| project.funder.name | Generalitat Valenciana | ca_CA |
| project.funder.name | Ministerio de Ciencia e Innovación | ca_CA |
| project.funder.name | Ministry of Education, Youth and Sports of the Czech Republic | ca_CA |
| project.funder.name | APOSTD/2021/251 | ca_CA |
| oaire.awardNumber | 2022R1A6A3A03068188 | ca_CA |
| oaire.awardNumber | 2022R1A2C1008252 | ca_CA |
| oaire.awardNumber | CIPROM/2021/078 | ca_CA |
| oaire.awardNumber | MFA/2022/020 | ca_CA |
| oaire.awardNumber | MCIN/PEICTI2021-2023/PID2021-122960OA-I00 | ca_CA |
| oaire.awardNumber | MCIN/PEICTI2021-2023/TED2021-131600B–C31 | ca_CA |
| oaire.awardNumber | M 2018103 | ca_CA |
| oaire.awardNumber | LM2023037 | ca_CA |
| oaire.awardNumber | IJC2020-042618-I | ca_CA |
| dc.subject.ods | 7. Energia asequible y no contaminante | ca_CA |
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