Synthesis of a Double-Network Supramolecular Hydrogel by Having One Network Catalyse the Formation of the Second
Impacto
Scholar |
Otros documentos de la autoría: Singh, Nishant; Maity, Chandan; Zhang, Kai; Angulo-Pachón, César A.; van Esch, Jan; Eelkema, Rienk; Escuder, Beatriu
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Mostrar el registro completo del ítemcomunitat-uji-handle:10234/9
comunitat-uji-handle2:10234/7053
comunitat-uji-handle3:10234/8639
comunitat-uji-handle4:
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http://dx.doi.org/10.1002/chem.201605771 |
Metadatos
Título
Synthesis of a Double-Network Supramolecular Hydrogel by Having One Network Catalyse the Formation of the SecondAutoría
Fecha de publicación
2017-02-10Editor
WileyISSN
0947-6539; 1521-3765Cita bibliográfica
SINGH, Nishant, et al. Synthesis of a Double‐Network Supramolecular Hydrogel by Having One Network Catalyse the Formation of the Second. Chemistry-A European Journal, 2017, vol. 23, no 9, p. 2018-2021.Tipo de documento
info:eu-repo/semantics/articleVersión de la editorial
http://onlinelibrary.wiley.com/doi/10.1002/chem.201605771/fullVersión
info:eu-repo/semantics/publishedVersionPalabras clave / Materias
Resumen
elf-assembly of biomolecules catalytically controls the formation of natural supramolecular structures, giving highly ordered complex materials. Such desirable hybrid systems are very difficult to design and construct ... [+]
elf-assembly of biomolecules catalytically controls the formation of natural supramolecular structures, giving highly ordered complex materials. Such desirable hybrid systems are very difficult to design and construct synthetically. A hybrid double-network hydrogel with a maximum storage modulus (G′max) of up to 55 kPa can be synthesized by using a self-assembled hydrogel that catalyses the formation of another kinetically arrested hydrogel network. Tuning of the catalytic efficiency of the first network allowed spatiotemporal control over the evolution of the second network and the resulting mechanical properties. The distribution of active catalytic sites was optimal for catalytic fibres prepared at the minimum gelation concentration (MGC) to give the double-network hydrogel with highest storage modulus. This approach could be very useful in preparing complex hierarchical structures with tailor-made properties. [-]
Publicado en
Chemistry-A European Journal, 2017, vol. 23, no 9, p. 2018-2021Proyecto de investigación
EU (Marie Curie ITN-Smartnet) / PITN-GA-2012316656Derechos de acceso
Copyright © John Wiley & Sons, Inc.
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