Multifunctional heterogeneous catalysts for the tandem CO2 hydrogenation-Fischer Tropsch synthesis of gasoline
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Title
Multifunctional heterogeneous catalysts for the tandem CO2 hydrogenation-Fischer Tropsch synthesis of gasolineDate
2022-09-15Publisher
ElsevierISSN
2212-9820Bibliographic citation
Martín, N., & Cirujano, F. G. (2022). Multifunctional heterogeneous catalysts for the tandem CO2 hydrogenation-Fischer Tropsch synthesis of gasoline. Journal of CO2 Utilization, 65, 102176.Type
info:eu-repo/semantics/articleVersion
info:eu-repo/semantics/acceptedVersionSubject
Abstract
The design of novel catalysts for the direct transformation of CO2 into gasoline is a promising valorization strategy for renewable liquid fuels. However, this process is highly challenging given the inertness of CO2 ... [+]
The design of novel catalysts for the direct transformation of CO2 into gasoline is a promising valorization strategy for renewable liquid fuels. However, this process is highly challenging given the inertness of CO2 and the thermodynamic limitations of its selective hydrogenation into C5+ hydrocarbons over more favored CH4 or CO byproducts. Thus, active, selective and stable multifunctional heterogeneous catalysts are needed in order to promote both the dissociative CO2 chemisorption and chain growth of the CHx species at the solid-gas interface under mild conditions (T < 400 °C, P < 50 bar). Several iron-containing multifunctional catalysts based on metal oxides, carbon or zeolite materials are reviewed here, discussing their preparation, characterization and catalytic performance in this environmentally and industrially relevant application, proposing future directions of the field. [-]
Is part of
Journal of CO2 Utilization. Volume 65, November 2022, 102176Funder Name
”la Caixa” Foundation | “Ramon y Cajal” Foundation | Juan de la Cierva formación
Project code
LCF/BQ/PI19/11690011 | RYC2020-028681-I | FJC2018-035455-I
Rights
2212-9820/© 2022 Published by Elsevier Ltd.
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