AuNP−polymeric ionic liquid composite multicatalytic nanoreactors for one-pot cascade reactions
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http://dx.doi.org/10.1021/acscatal.6b01759 |
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Título
AuNP−polymeric ionic liquid composite multicatalytic nanoreactors for one-pot cascade reactionsAutoría
Fecha de publicación
2016Editor
American Chemical SocietyISSN
2155-5435Tipo de documento
info:eu-repo/semantics/articleVersión de la editorial
http://pubs.acs.org/doi/abs/10.1021/acscatal.6b01759Palabras clave / Materias
Resumen
Different AuNP-PIL nanocomposites have been developed
as bifunctional catalysts in which the IL-like units promote the Knoevenagel
condensation through a dual electrophilic/nucleophilic activation relay
mechanism ... [+]
Different AuNP-PIL nanocomposites have been developed
as bifunctional catalysts in which the IL-like units promote the Knoevenagel
condensation through a dual electrophilic/nucleophilic activation relay
mechanism and metal nanoparticles catalyze the reduction of the functional
groups of the Knoevenagel product in a one-pot tandem reaction. The
characterization of the composites by different techniques suggests that the
self-assembly and self-organization of the constituent building blocks during
the synthetic procedures define the precise shapes, sizes, and catalytic
performance of these advanced materials. The resulting catalytic efficiency
reflects not only the presence of the corresponding individual catalytic
motifs but also their hierarchical organization. [-]
Publicado en
ACS Catal. 2016, 6, 7230−7237Derechos de acceso
© 2016 American Chemical Society
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