AuNP−polymeric ionic liquid composite multicatalytic nanoreactors for one-pot cascade reactions
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Show full item recordcomunitat-uji-handle:10234/9
comunitat-uji-handle2:10234/7053
comunitat-uji-handle3:10234/8639
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http://dx.doi.org/10.1021/acscatal.6b01759 |
Metadata
Title
AuNP−polymeric ionic liquid composite multicatalytic nanoreactors for one-pot cascade reactionsAuthor (s)
Date
2016Publisher
American Chemical SocietyISSN
2155-5435Type
info:eu-repo/semantics/articlePublisher version
http://pubs.acs.org/doi/abs/10.1021/acscatal.6b01759Subject
Abstract
Different AuNP-PIL nanocomposites have been developed
as bifunctional catalysts in which the IL-like units promote the Knoevenagel
condensation through a dual electrophilic/nucleophilic activation relay
mechanism ... [+]
Different AuNP-PIL nanocomposites have been developed
as bifunctional catalysts in which the IL-like units promote the Knoevenagel
condensation through a dual electrophilic/nucleophilic activation relay
mechanism and metal nanoparticles catalyze the reduction of the functional
groups of the Knoevenagel product in a one-pot tandem reaction. The
characterization of the composites by different techniques suggests that the
self-assembly and self-organization of the constituent building blocks during
the synthetic procedures define the precise shapes, sizes, and catalytic
performance of these advanced materials. The resulting catalytic efficiency
reflects not only the presence of the corresponding individual catalytic
motifs but also their hierarchical organization. [-]
Is part of
ACS Catal. 2016, 6, 7230−7237Rights
© 2016 American Chemical Society
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