Towards highly efficient continuous-flow catalytic carbon dioxide cycloadditions with additively manufactured reactors
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Otros documentos de la autoría: Valverde Barquero, David; Porcar Garcia, Raul; Zanatta, Marcileia; Alcalde, Sergio; Altava, Belen; Sans, Victor; Garcia-Verdugo, Eduardo
Metadatos
Mostrar el registro completo del ítemcomunitat-uji-handle:10234/9
comunitat-uji-handle2:10234/160292
comunitat-uji-handle3:10234/160293
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INVESTIGACIONMetadatos
Título
Towards highly efficient continuous-flow catalytic carbon dioxide cycloadditions with additively manufactured reactorsAutoría
Fecha de publicación
2022-03-22Editor
The Royal Society of ChemistryISSN
1463-9270Cita bibliográfica
VALVERDE, David, et al. Towards highly efficient continuous-flow catalytic carbon dioxide cycloadditions with additively manufactured reactors. Green Chemistry, 2022.Tipo de documento
info:eu-repo/semantics/articleVersión de la editorial
https://pubs.rsc.org/en/content/articlelanding/2022/gc/d1gc04593hVersión
info:eu-repo/semantics/acceptedVersionResumen
Developing efficient and sustainable methodologies to transform CO2 into added-value chemicals is an important strategy for decarbonization in the chemical industry. Here, a new multi-scale approach for the cycloaddition ... [+]
Developing efficient and sustainable methodologies to transform CO2 into added-value chemicals is an important strategy for decarbonization in the chemical industry. Here, a new multi-scale approach for the cycloaddition of CO2 to epoxides is reported, designed by combining the hydrogen bonding ability, metal-free catalysts and supported ionic liquids on polymers. The use of additive manufacturing (AM) techniques allowed the digital design and rapid fabrication of structured architectures for continuous-flow reactors, which offers potential for process optimization. AM generated catalytic reactors showed higher catalytic activity than similar sized packed bed reactors, when normalised to the amount of catalyst and their surface area. The catalytic activity and stability were maintained over a prolonged period of time (300 h) without loss of activity, and it was demonstrated to efficiently transform a range of epoxide substrates. [-]
Publicado en
Green Chemistry, 2022Entidad financiadora
Universitat Jaume I | Ministerio de Ciencia e Innovación | Agencia Estatal de Investigación | FEDER | Generalitat Valenciana | European Union's Horizon 2020 | Marie Skłodowska-Curie Individual Fellowships
Código del proyecto o subvención
UJI-B2019-40 | UJI-B2020-44 | RTI2018-098233-B-C22 | RTI2018-098233-B-C21 | H2020-MSCA-IF-101026335 | CIDEGENT 2018/036
Proyecto de investigación
info:eu-repo/grantAgreement/EC/H2020/101026335Derechos de acceso
http://rightsstatements.org/vocab/InC/1.0/
info:eu-repo/semantics/openAccess
info:eu-repo/semantics/openAccess
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