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Insight into Copper-Based Catalysts: Microwave-Assisted Morphosynthesis, In Situ Reduction Studies, and Dehydrogenation of Ethanol

dc.contributor.authorVolanti, Diogo P.
dc.contributor.authorSato, André G.
dc.contributor.authorOrlandi, Marcelo
dc.contributor.authorBueno, José M. C.
dc.contributor.authorLongo, Elson
dc.contributor.authorAndres, Juan
dc.date.accessioned2017-04-06T11:10:18Z
dc.date.available2017-04-06T11:10:18Z
dc.date.issued2011
dc.identifier.citationVolanti, D. P., Sato, A. G., Orlandi, M. O., Bueno, J. M. C., Longo, E. and Andrés, J. (2011), Insight into Copper-Based Catalysts: Microwave-Assisted Morphosynthesis, In Situ Reduction Studies, and Dehydrogenation of Ethanol. ChemCatChem, 3: 839–843. doi:10.1002/cctc.201000462ca_CA
dc.identifier.issn1867-3880
dc.identifier.urihttp://hdl.handle.net/10234/167154
dc.description.abstractCopper-based catalysts obtained by microwave-assisted morphosynthesis were correlated with the dehydrogenation of ethanol. The degree of reduction was monitored using time-resolved in situ XANES during TPR under H2. A semiquantitative estimation of the different chemical forms (Cu2+, Cu+, and/or Cu0) was obtained. The results suggest intrinsic particularities due to different morphologies at the active state in reduction kinetics.ca_CA
dc.description.sponsorShipWe would like to thank the CNPq, FAPESP and Ministerio de Cien- cia y Tecnologia (Spain) and the Spanish–Brazilian program (PHB2009-0065-PC) for their financial support. The XANES facili- ties were supplied by LNLS (National Laboratory of Synchrotron Light, Brazil) Beamline (D06A-DXAS-10156) and TEM facilities by LME-LNLS.ca_CA
dc.format.extent5 p.ca_CA
dc.format.mimetypeapplication/pdfca_CA
dc.language.isoengca_CA
dc.publisherWileyca_CA
dc.relation.isPartOfChemCatChem, 2011, 3ca_CA
dc.rightsCopyright 2011 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheimca_CA
dc.rights.urihttp://rightsstatements.org/vocab/InC/1.0/*
dc.subjectcopperca_CA
dc.subjectdehydrogenationca_CA
dc.subjectmicrowave chemistryca_CA
dc.subjectreductionca_CA
dc.subjectX-ray absorption spectroscopyca_CA
dc.titleInsight into Copper-Based Catalysts: Microwave-Assisted Morphosynthesis, In Situ Reduction Studies, and Dehydrogenation of Ethanolca_CA
dc.typeinfo:eu-repo/semantics/articleca_CA
dc.identifier.doihttp://dx.doi.org/10.1002/cctc.201000462
dc.rights.accessRightsinfo:eu-repo/semantics/restrictedAccessca_CA
dc.relation.publisherVersionhttp://onlinelibrary.wiley.com/doi/10.1002/cctc.201000462/abstractca_CA
dc.type.versioninfo:eu-repo/semantics/publishedVersion


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