An Experimental and Computational Study of β-AgVO3: Optical Properties and Formation of Ag Nanoparticles
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Altres documents de l'autoria: Oliveira, Regiane; Assis, Marcelo de; Teixeira, Mayara Mondego; Penha da Silva, Maya Dayana; Siu Li, Maximo; Andres, Juan; Gracia, Lourdes; Longo, Elson
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Mostra el registre complet de l'elementcomunitat-uji-handle:10234/9
comunitat-uji-handle2:10234/7013
comunitat-uji-handle3:10234/8638
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An Experimental and Computational Study of β-AgVO3: Optical Properties and Formation of Ag NanoparticlesAutoria
Data de publicació
2016-05-19Editor
ACS PublicationsISSN
1932-7447Cita bibliogràfica
OLIVEIRA, Regiane Cristina de, et al. An Experimental and Computational Study of β-AgVO3: Optical Properties and Formation of Ag Nanoparticles. The Journal of Physical Chemistry C, 2016Tipus de document
info:eu-repo/semantics/articleVersió de l'editorial
http://pubs.acs.org/doi/abs/10.1021/acs.jpcc.6b02840Versió
info:eu-repo/semantics/submittedVersionParaules clau / Matèries
Resum
This article aims to gather together in one place and for first time the formation process of Ag nanoparticles (NPs) on β-AgVO3 crystals, driven by an accelerated electron beam from an electronic microscope under high ... [+]
This article aims to gather together in one place and for first time the formation process of Ag nanoparticles (NPs) on β-AgVO3 crystals, driven by an accelerated electron beam from an electronic microscope under high vacuum. Synthesis and optical properties of β-AgVO3 are reported, and the relationship between structural disorder and photoluminescence emissions is discussed. First principle calculations, within a QTAIM framework, have been carried out to provide a deeper insight and understanding of the observed nucleation and early evolution of Ag nanoparticles (NPs) on β-AgVO3 crystals. The Ag nucleation and formation is a result of structural and electronic changes of the [AgO5] and [AgO6] clusters, consistent with Ag metallic formation. [-]
Publicat a
The Journal of Physical Chemistry C, 2016, vol. 120, n. 22Drets d'accés
Copyright © 2016 American Chemical Society
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info:eu-repo/semantics/openAccess
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