Listar por autoría "88694efd-397f-4218-8a50-621b64f30adf"
Mostrando ítems 41-60 de 70
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Hole spin relaxation in InAS/GaAs quantum dot molecules
Segarra, Carlos; Climente, Juan I.; Rajadell Viciano, Fernando; Planelles, Josep IOP Publishing Ltd (2015-09)We calculate the spin–orbit induced hole spin relaxation between Zeeman sublevels of vertically stacked InAs quantum dots. The widely used Luttinger–Kohn Hamiltonian, which considers coupling of heavy- and light-holes, ... -
Influence of Polytypism on the Electronic Structure of CdSe/CdS and CdSe/CdSe Core/Shell Nanocrystals
Segarra, Carlos; Rajadell Viciano, Fernando; Climente, Juan I.; Planelles, Josep American Chemical Society (2017-03)We address theoretically differences and similarities on the electronic structure of CdSe/CdS dot-in-dot nanocrystals (NCs) with wurtzite/wurtzite (WZ/WZ), zinc-blende/zinc-blende (ZB/ZB) and polytype ZB/WZ crystalline ... -
Large hole spin anticrossings in InAs/GaAs double quantum dots
Rajadell Viciano, Fernando; Planelles, Josep; Climente, Juan I. AIP Publishing (2013-09-23)We show that hole states in InAs/GaAs double quantum dots can exhibit spin anticrossings of up to 1 meV, according to simulations with a three dimensional Burt-Foreman Hamiltonian including strain and piezoelectric fields. ... -
Large-scale linear system solver using secondary storage: self-energy in hybrid nanostructures
Badía, José; Movilla, Jose L.; Climente, Juan I.; Castillo Catalán, María Isabel; Marqués-Andrés, Mercedes; Mayo, Rafael; Quintana-Orti, Enrique S.; Planelles, Josep Elsevier (2011-02)We present a Fortran library which can be used to solve large-scale dense linear systems, Ax=b. The library is based on the LU decomposition included in the parallel linear algebra library PLAPACK and on its out-of-core ... -
Magnetic field implementation in multiband k⋅p Hamiltonians of holes in semiconductor heterostructures
Planelles, Josep; Climente, Juan I. IOP Publishing (2013) -
Morphology and Band Structure of Orthorhombic PbS Nanoplatelets: An Indirect Band Gap Material
Macias-Pinilla, David F.; Echeverría-Arrondo, Carlos; Gualdrón Reyes, Andrés Fabián; Agouram, Said; Muñoz-Sanjosé, Vicente; Planelles, Josep; Mora-Sero, Ivan; Climente, Juan I. American Chemical Society (2021-01-12)PbS quantum dots and nanoplatelets (NPLs) are of enormous interest in the development of optoelectronic devices. However, some important aspects of their nature remain unclear. Recent studies have revealed that colloidal ... -
Nature and Control of Shakeup Processes in Colloidal Nanoplatelets
Llusar, Jordi; Climente, Juan I. American Chemical Society (2020-10-29)Recent experiments suggest that the photoluminescence line width of CdSe nanoplatelets (NPLs) and core/shell CdSe/CdS NPLs may be broadened by the presence of shakeup (SU) lines from negatively charged trions. We carry ... -
One- and Two-Photon Absorption in CdS Nanodots and Wires: The Role of Dimensionality in the One- and Two-Photon Luminescence Excitation Spectrum
Achtstein, Alexander W.; Ballester Caudet, Ana; Movilla, Jose L.; Hennig, Jonas; Climente, Juan I.; Prudnikau, Anatol V.; Antanovich, Artsiom; Scott, Riccardo; Artemyev, Mikhail V.; Planelles, Josep; Woggon, Ulrike American Chemical Society (2014-12)We investigate the spectral dependence of the linear and two-photon absorption of wurtzite CdS nanoparticles (dots and rods) by means of quantitative one- and two-photon photoluminescence excitation spectroscopy and effective ... -
Optimized Cation Exchange for Mercury Chalcogenide 2D Nanoplatelets and Its Application for Alloys
Dabard, Corentin; Planelles, Josep; Po, Hong; Izquierdo, Eva; Makke, Lina; Gréboval, Charlie; Moghaddam, Nicolas; Khalili Lazarjani, Adrien; Dang Huu, Tung; Chu, Audrey; Pierini, Stefano; Abadie, Claire; Cavallo, Mariarosa; Bossavit, Erwan; Xu, XiangXiang Zhen; Hollander, Philippe; Silly, Mathieu; Lhuillier, Emmanuel; Climente, Juan I.; Ithurria, Sandrine American Chemical Society (2021-11-29)II–VI two-dimensional (2D) nanoplatelets (NPLs) exhibit the narrowest optical features among nanocrystals (NCs). This property remains true for Hg-based NPLs, despite a cation exchange procedure to obtain them from Cd-based ... -
Origin of electron spin-orbit anisotropy in pyramidal InAs quantum dots
Segarra, Carlos; Planelles, Josep; Climente, Juan I. Elsevier (2015)We investigate the electron spin–orbit interaction anisotropy of pyramidal InAs quantum dots using a fully three-dimensional Hamiltonian. The dependence of the spin–orbit interaction strength on the orientation of externally ... -
Origin of two-hole triplet splitting in circular quantum dots
Climente, Juan I. Elsevier (2012-05)Recent photoluminescence spectra of positively charged excitons in InAs/GaAs quantum dots have revealed the existence of large splittings between the View the MathML sourcep-shell triplet sublevels of holes. We provide an ... -
Photoluminescence spectroscopy of trions in quantum dots: A theoretical description
Goldoni, Guido; Bertoni, Andrea; Climente, Juan I. American Physical Society (2008)We present a full configuration-interaction study of the spontaneous recombination of neutral and singly charged excitons trions in semiconductor quantum dots from weak- to strong-coupling regimes. We find that the ... -
Piezoelectric Control of the Exciton Wave Function in Colloidal CdSe/CdS Nanocrystals
Segarra, Carlos; Climente, Juan I.; Polovitsyn, Anatolii; Rajadell Viciano, Fernando; Moreels, Iwan; Planelles, Josep American Chemical Society (2016-05-25)Using multiband k·p calculations, we show that strain-engineered piezoelectricity is a powerful tool to modulate the electron−hole spatial separation in a wide class of wurtzite CdSe/CdS nanocrystals. The inherent ... -
Role of alternance symmetry in magnetoconductance
Planelles, Josep; Climente, Juan I. American Physical Society (2014)We show that the direction of coherent electron transport across a cyclic system of quantum dots or a cyclic molecule can be modulated by an external magnetic field if the cycle has an odd number of hopping sites, but the ... -
Role of thermally occupied hole states in room-temperature broadband gain in CdSe/CdS giant-shell nanocrystals
Tanghe, Ivo; Llusar, Jordi; Climente, Juan I.; Barker, Alex J.; Paternò, Giuseppe Maria; Scotognella, Francesco; Polovitsyn, Anatolii; Khan, Ali Hossain; hens, zeger; Van Thourhout, Dries; Geiregat, Pieter; Moreels, Iwan Wiley (2022)Growing CdSe/CdS nanocrystals from a large CdSe core, and employing a giant CdS shell, a continuous, broadband gain spectrum, covering the spectral range between the CdSe and the CdS band edge, is induced. As revealed by ... -
Scalable qubit architecture based on holes in quantum dot molecules
Economou, Sophia E.; Climente, Juan I.; Badolato, Antonio; Bracker, Allan S.; Gammon, Daniel; Doty, Matthew F. American Physical Society (2012)Spins confined in quantum dots are a leading candidate for solid-state quantum bits that can be coherently controlled by optical pulses. There are, however, many challenges to developing a scalable multibit information ... -
Shell filling and paramagnetism in few-electron colloidal nanoplatelets
Llusar, Jordi; Climente, Juan I. American Physical Society (2022-08-05)Colloidal semiconductor nanoplatelets are excellent optical emitters, which combine a quasi-2D structure with strong in-plane Coulomb interactions. Here, we go beyond the photoexcitation regime and investigate theoretically ... -
Spin–orbit-induced hole spin relaxation in InAs and GaAs quantum dots
Climente, Juan I.; Segarra, Carlos; Planelles, Josep Institute of Physics (2013)We study the effect of valence band spin–orbit interactions (SOI) on the acoustic phonon-assisted spin relaxation of holes confined in quantum dots (QDs). Heavy hole–light hole (hh–lh) mixing and all the spin–orbit terms ... -
Strain in Lattice-Mismatched CdSe-Based Core/Shell Nanoplatelets
Llusar, Jordi; Planelles, Josep; Climente, Juan I. American Chemical Society (2019-08-05)We investigate the role of stress arising between core and shell materials in colloidal CdSe/X hetero-nanoplatelets (X = ZnS, CdS, CdTe). The resulting strain distribution is calculated within the linear elastic regime and ... -
Strong configuration mixing due to dielectric confinement in semiconductor nanorods
Climente, Juan I.; Royo Valls, Miguel; Movilla, Jose L.; Planelles, Josep American Physical Society (2009)The interaction between electron-electron and electron-hole pairs in semiconductor nanorods embedded in dielectric media is investigated using a configuration-interaction method. Contrary to spherical quantum dots of similar ...