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Tandem Catalysis of an Aldol-'Click' Reaction System within a Molecular Hydrogel
dc.contributor.author | Araujo, Marco | |
dc.contributor.author | Muñoz Capdevila, Iván | |
dc.contributor.author | Diaz-Oltra, Santiago | |
dc.contributor.author | Escuder, Beatriu | |
dc.date.accessioned | 2016-07-29T07:22:07Z | |
dc.date.available | 2016-07-29T07:22:07Z | |
dc.date.issued | 2016-06 | |
dc.identifier.citation | ARAÚJO, Marco, et al. Tandem Catalysis of an Aldol-‘Click’Reaction System within a Molecular Hydrogel. Molecules, 2016, vol. 21, no 6, p. 744. | ca_CA |
dc.identifier.uri | http://hdl.handle.net/10234/162064 | |
dc.description.abstract | A heterogeneous supramolecular catalytic system for multicomponent aldol-‘click’ reactions is reported. The copper(I) metallohydrogel functionalized with a phenyltriazole fragment was able to catalyze the multicomponent reaction between phenylacetylene, p-nitrobenzaldehyde, and an azide containing a ketone moiety, obtaining the corresponding aldol products in good yields. A possible mechanistic pathway responsible for this unexpected catalytic behavior has been proposed. | ca_CA |
dc.description.sponsorShip | This work was supported by the EU (Marie Curie ITN-Smartnet, Grant PITN-GA- 2012-316656). M. A. thanks EU for an ESR Marie Curie contract. | ca_CA |
dc.format.extent | 13 p. | ca_CA |
dc.format.mimetype | application/pdf | ca_CA |
dc.language.iso | eng | ca_CA |
dc.publisher | MDPI | ca_CA |
dc.relation.isPartOf | Molecules 2016, 21(6) | ca_CA |
dc.rights | © 1996-2016 MDPI AG (Basel, Switzerland) unless otherwise stated | ca_CA |
dc.rights | Atribución 4.0 España | * |
dc.rights.uri | http://creativecommons.org/licenses/by-sa/4.0/ | * |
dc.subject | aldol addition | ca_CA |
dc.subject | click reaction | ca_CA |
dc.subject | tandem catalysis | ca_CA |
dc.subject | supramolecular gels | ca_CA |
dc.subject | multicomponent system | ca_CA |
dc.title | Tandem Catalysis of an Aldol-'Click' Reaction System within a Molecular Hydrogel | ca_CA |
dc.type | info:eu-repo/semantics/article | ca_CA |
dc.identifier.doi | http://dx.doi.org/10.3390/molecules21060744 | |
dc.rights.accessRights | info:eu-repo/semantics/openAccess | ca_CA |
dc.relation.publisherVersion | http://www.mdpi.com/1420-3049/21/6/744 | ca_CA |
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